But, by Monday, the glamour was a distant memory as the mother-of-six reverted back to her parental duties.
The 33-year-old actress took half of her extensive brood out for an afternoon stroll to the shops in New Orleans yesterday.
Walk about: Angelina Jolie takes three of her six children Shiloh, Pax and Zahara for a walk to a nearby store in New Orleans yesterday
Leaving three-month-old twins Vivienne and Knox at home with their seven-year-old brother Maddox, Angelina brought Pax Thien, four; Zahara Marley, three; and Shiloh Nouvel, two; to the local Verdi Mart.
Dressed in a floor-length black dress, Angelina was careful not to trip as she carried blonde haired Shiloh, who was clutching her beloved pink blankie and wearing neon green Crocs.
With mum Angelina going for the feminine look in her gown, tomboys Shiloh and Zahara were dressed in coloured jeans, while big brother Pax went for the workmen-style in dungarees.
The cute quartet, closely followed by two security guards, stopped into the store to buy packets of Cheetos (cheese-flavoured cornmeal snack) for the kids and some bottled water.
Snack time: The kids clutch their bags of Cheetos after mum Angelina brought them to a local store
Earlier that day, proud father Brad was spotted cycling around the city on the way to a business lunch at Creole restaurant Antoine's.
Wearing a fedora hat instead of a cycling helmet, the handsome star was clutching a notebook with a picture of U.S. Presidential candidate Barack Obama on it.
The superstar couple bought a £1.75million, six bedroomed 1830s house in New Orleans' historic French Quarter in early 2007 in a bid to help regenerate the area.
The couple have spent time and money helping rebuilding the Louisiana city following the devastation caused by Hurricane Katrina in 2005.
Apple of my eye: Angelina keeps an eye on two-year-old Shiloh as she carries her pink blankie
They returned to New Orleans on Monday for the first time since the Spring after spending the weekend in New York.
The couple have spent most of the year in Europe - renting the £35million Miraval Estate villa in the French hamlet of Correns, in the Provence region, before moving to Germany last month, where Brad is expected to remain for most of the year filming his latest movie.
Angelina made her first public appearance since the birth of the twins on July 12th at the Big Apple screening of her new film The Changeling.
Showing support: Brad Pitt cycles to a business lunch clutching a notebook with a picture of Barack Obama
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